The word(s) "devote" appears 4 time(s) in 4 verse(s) in Quran in Muhammad Pickthal translation.

(1) And with how many a prophet have there been a number of devoted men who fought (beside him). They quailed not for aught that befell them in the way of Allah, nor did they weaken, nor were they brought low. Allah loveth the steadfast.

(سورة آل عمران, Aal-i-Imraan, Chapter #3, Verse #146)
(Arabic, Transliteration, Urdu (Ahmed Ali), Urdu (Jalandhry), Farsi, Yusuf Ali, Shakir, Picthal, Mohsin Khan, French, Spanish, Indonesian, Malay, German, Bosnian, Russian, Dutch, Italian, Portuguese, Tafsir - Jalal ad-Din, Tafsir - King Fahad Quran Complex)

(2) Save such of them as are Thy perfectly devoted slaves.

(سورة الحجر, Al-Hijr, Chapter #15, Verse #40)
(Arabic, Transliteration, Urdu (Ahmed Ali), Urdu (Jalandhry), Farsi, Yusuf Ali, Shakir, Picthal, Mohsin Khan, French, Spanish, Indonesian, Malay, German, Bosnian, Russian, Dutch, Italian, Portuguese, Tafsir - Jalal ad-Din, Tafsir - King Fahad Quran Complex)

(3) They said: We worship idols, and are ever devoted unto them.

(سورة الشعراء, Ash-Shu'araa, Chapter #26, Verse #71)
(Arabic, Transliteration, Urdu (Ahmed Ali), Urdu (Jalandhry), Farsi, Yusuf Ali, Shakir, Picthal, Mohsin Khan, French, Spanish, Indonesian, Malay, German, Bosnian, Russian, Dutch, Italian, Portuguese, Tafsir - Jalal ad-Din, Tafsir - King Fahad Quran Complex)

(4) So remember the name of thy Lord and devote thyself with a complete devotion -

(سورة المزمل, Al-Muzzammil, Chapter #73, Verse #8)
(Arabic, Transliteration, Urdu (Ahmed Ali), Urdu (Jalandhry), Farsi, Yusuf Ali, Shakir, Picthal, Mohsin Khan, French, Spanish, Indonesian, Malay, German, Bosnian, Russian, Dutch, Italian, Portuguese, Tafsir - Jalal ad-Din, Tafsir - King Fahad Quran Complex)